Sorption and transport of sulfamethazine in agricultural soils amended with invasive-plant-derived biochar.
Identifieur interne : 000335 ( Main/Exploration ); précédent : 000334; suivant : 000336Sorption and transport of sulfamethazine in agricultural soils amended with invasive-plant-derived biochar.
Auteurs : Meththika Vithanage [Sri Lanka] ; Anushka Upamali Rajapaksha [Sri Lanka] ; Xiangyu Tang [République populaire de Chine] ; Sören Thiele-Bruhn [Allemagne] ; Kye Hoon Kim [Corée du Sud] ; Sung-Eun Lee [Corée du Sud] ; Yong Sik Ok [Canada]Source :
- Journal of environmental management [ 1095-8630 ] ; 2014.
English descriptors
- KwdEn :
- MESH :
- chemical , analysis : Anti-Bacterial Agents, Soil Pollutants, Sulfamethazine.
- chemical , chemistry : Anti-Bacterial Agents, Soil Pollutants, Sulfamethazine.
- methods : Waste Management.
- Adsorption, Agriculture, Charcoal, Cucurbitaceae, Introduced Species, Temperature.
Abstract
Sulfonamides (SAs) are one of the most frequently used antibiotics in the veterinary industry, showing high mobility in soils. Objectives of this research were to determine the sorption, distribution coefficients and involvement of different ionic forms of sulfamethazine (SMZ), a representative SAs, and to evaluate the transport of SMZ in biochar treated soils. Biochars were produced from an invasive plant, burcucumber (Sicyos angulatus L.), under slow pyrolysis conditions at peak temperatures of 300 °C (biochar-300) and 700 °C (biochar-700), respectively. The abilities of the biochars to retain SMZ in loamy sand and sandy loam soils were examined under different pHs and SMZ loadings. Soil column experiments were performed with and without biochars addition. Results showed that biochar-700 had a high degree of SMZ retention, with resultant decreased pH in both soils. Modeled effective sorption coefficients (KD,eff) values indicated that the observed high SMZ retention at pH 3 could be attributed to the π-π electron donor-acceptor interaction and electrostatic cation exchange, whereas at pH 5 and 7, cation exchange was the main mechanisms responsible. There was no temporal retardation of SMZ in biochar treated soil as compared to the untreated soil. However, biochar-700 treatment achieved up to 89% and 82% increase in the SMZ retention in sandy loam and loamy sand soils, respectively. The overall results demonstrated that burcucumber biochar produced at higher temperature was effective in reducing the mobility of SMZ in the studied soils.
DOI: 10.1016/j.jenvman.2014.02.030
PubMed: 24768839
Affiliations:
- Allemagne, Canada, Corée du Sud, République populaire de Chine, Sri Lanka
- Rhénanie-Palatinat
- Séoul, Trèves (Allemagne)
- Université de Trèves
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Le document en format XML
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Electronic address: soilok@kangwon.ac.kr.</nlm:affiliation><country xml:lang="fr">Canada</country><wicri:regionArea>Korea Biochar Research Center and Department of Biological Environment, Kangwon National University, Chuncheon, Republic of Korea; Department of Renewable Resources, University of Alberta, Edmonton</wicri:regionArea><wicri:noRegion>Edmonton</wicri:noRegion></affiliation></author></titleStmt><publicationStmt><idno type="wicri:source">PubMed</idno><date when="2014">2014</date><idno type="RBID">pubmed:24768839</idno><idno type="pmid">24768839</idno><idno type="doi">10.1016/j.jenvman.2014.02.030</idno><idno type="wicri:Area/PubMed/Corpus">000346</idno><idno type="wicri:explorRef" wicri:stream="PubMed" wicri:step="Corpus" wicri:corpus="PubMed">000346</idno><idno type="wicri:Area/PubMed/Curation">000346</idno><idno type="wicri:explorRef" wicri:stream="PubMed" wicri:step="Curation">000346</idno><idno type="wicri:Area/PubMed/Checkpoint">000346</idno><idno type="wicri:explorRef" wicri:stream="Checkpoint" wicri:step="PubMed">000346</idno><idno type="wicri:Area/Ncbi/Merge">000676</idno><idno type="wicri:Area/Ncbi/Curation">000676</idno><idno type="wicri:Area/Ncbi/Checkpoint">000676</idno><idno type="wicri:Area/Main/Merge">000336</idno><idno type="wicri:Area/Main/Curation">000335</idno><idno type="wicri:Area/Main/Exploration">000335</idno></publicationStmt><sourceDesc><biblStruct><analytic><title xml:lang="en">Sorption and transport of sulfamethazine in agricultural soils amended with invasive-plant-derived biochar.</title><author><name sortKey="Vithanage, Meththika" sort="Vithanage, Meththika" uniqKey="Vithanage M" first="Meththika" last="Vithanage">Meththika Vithanage</name><affiliation wicri:level="1"><nlm:affiliation>Korea Biochar Research Center and Department of Biological Environment, Kangwon National University, Chuncheon, Republic of Korea; Chemical and Environmental Systems Modeling Research Group, Institute of Fundamental Studies, Kandy, Sri Lanka.</nlm:affiliation><country xml:lang="fr">Sri Lanka</country><wicri:regionArea>Korea Biochar Research Center and Department of Biological Environment, Kangwon National University, Chuncheon, Republic of Korea; Chemical and Environmental Systems Modeling Research Group, Institute of Fundamental Studies, Kandy</wicri:regionArea><wicri:noRegion>Kandy</wicri:noRegion></affiliation></author><author><name sortKey="Rajapaksha, Anushka Upamali" sort="Rajapaksha, Anushka Upamali" uniqKey="Rajapaksha A" first="Anushka Upamali" last="Rajapaksha">Anushka Upamali Rajapaksha</name><affiliation wicri:level="1"><nlm:affiliation>Korea Biochar Research Center and Department of Biological Environment, Kangwon National University, Chuncheon, Republic of Korea; Chemical and Environmental Systems Modeling Research Group, Institute of Fundamental Studies, Kandy, Sri Lanka.</nlm:affiliation><country xml:lang="fr">Sri Lanka</country><wicri:regionArea>Korea Biochar Research Center and Department of Biological Environment, Kangwon National University, Chuncheon, Republic of Korea; Chemical and Environmental Systems Modeling Research Group, Institute of Fundamental Studies, Kandy</wicri:regionArea><wicri:noRegion>Kandy</wicri:noRegion></affiliation></author><author><name sortKey="Tang, Xiangyu" sort="Tang, Xiangyu" uniqKey="Tang X" first="Xiangyu" last="Tang">Xiangyu Tang</name><affiliation wicri:level="1"><nlm:affiliation>Institute of Mountain Hazards and Environment, Chinese Academy of Sciences, Chengdu, China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Institute of Mountain Hazards and Environment, Chinese Academy of Sciences, Chengdu</wicri:regionArea><wicri:noRegion>Chengdu</wicri:noRegion></affiliation></author><author><name sortKey="Thiele Bruhn, Soren" sort="Thiele Bruhn, Soren" uniqKey="Thiele Bruhn S" first="Sören" last="Thiele-Bruhn">Sören Thiele-Bruhn</name><affiliation wicri:level="4"><nlm:affiliation>Department of Soil Science, University of Trier, Trier, Germany.</nlm:affiliation><country xml:lang="fr">Allemagne</country><wicri:regionArea>Department of Soil Science, University of Trier, Trier</wicri:regionArea><wicri:noRegion>Trier</wicri:noRegion><orgName type="university">Université de Trèves</orgName><placeName><settlement type="city">Trèves (Allemagne)</settlement><region type="land" nuts="1">Rhénanie-Palatinat</region></placeName></affiliation></author><author><name sortKey="Kim, Kye Hoon" sort="Kim, Kye Hoon" uniqKey="Kim K" first="Kye Hoon" last="Kim">Kye Hoon Kim</name><affiliation wicri:level="3"><nlm:affiliation>Department of Environmental Horticulture, The University of Seoul, Seoul, Republic of Korea.</nlm:affiliation><country xml:lang="fr">Corée du Sud</country><wicri:regionArea>Department of Environmental Horticulture, The University of Seoul, Seoul</wicri:regionArea><placeName><settlement type="city">Séoul</settlement></placeName></affiliation></author><author><name sortKey="Lee, Sung Eun" sort="Lee, Sung Eun" uniqKey="Lee S" first="Sung-Eun" last="Lee">Sung-Eun Lee</name><affiliation wicri:level="1"><nlm:affiliation>School of Applied Biosciences, Kyungpook National University, Daegu, Republic of Korea.</nlm:affiliation><country xml:lang="fr">Corée du Sud</country><wicri:regionArea>School of Applied Biosciences, Kyungpook National University, Daegu</wicri:regionArea><wicri:noRegion>Daegu</wicri:noRegion></affiliation></author><author><name sortKey="Ok, Yong Sik" sort="Ok, Yong Sik" uniqKey="Ok Y" first="Yong Sik" last="Ok">Yong Sik Ok</name><affiliation wicri:level="1"><nlm:affiliation>Korea Biochar Research Center and Department of Biological Environment, Kangwon National University, Chuncheon, Republic of Korea; Department of Renewable Resources, University of Alberta, Edmonton, Canada. Electronic address: soilok@kangwon.ac.kr.</nlm:affiliation><country xml:lang="fr">Canada</country><wicri:regionArea>Korea Biochar Research Center and Department of Biological Environment, Kangwon National University, Chuncheon, Republic of Korea; Department of Renewable Resources, University of Alberta, Edmonton</wicri:regionArea><wicri:noRegion>Edmonton</wicri:noRegion></affiliation></author></analytic><series><title level="j">Journal of environmental management</title><idno type="eISSN">1095-8630</idno><imprint><date when="2014" type="published">2014</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Adsorption</term><term>Agriculture</term><term>Anti-Bacterial Agents (analysis)</term><term>Anti-Bacterial Agents (chemistry)</term><term>Charcoal</term><term>Cucurbitaceae</term><term>Introduced Species</term><term>Soil Pollutants (analysis)</term><term>Soil Pollutants (chemistry)</term><term>Sulfamethazine (analysis)</term><term>Sulfamethazine (chemistry)</term><term>Temperature</term><term>Waste Management (methods)</term></keywords><keywords scheme="MESH" type="chemical" qualifier="analysis" xml:lang="en"><term>Anti-Bacterial Agents</term><term>Soil Pollutants</term><term>Sulfamethazine</term></keywords><keywords scheme="MESH" type="chemical" qualifier="chemistry" xml:lang="en"><term>Anti-Bacterial Agents</term><term>Soil Pollutants</term><term>Sulfamethazine</term></keywords><keywords scheme="MESH" qualifier="methods" xml:lang="en"><term>Waste Management</term></keywords><keywords scheme="MESH" xml:lang="en"><term>Adsorption</term><term>Agriculture</term><term>Charcoal</term><term>Cucurbitaceae</term><term>Introduced Species</term><term>Temperature</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">Sulfonamides (SAs) are one of the most frequently used antibiotics in the veterinary industry, showing high mobility in soils. Objectives of this research were to determine the sorption, distribution coefficients and involvement of different ionic forms of sulfamethazine (SMZ), a representative SAs, and to evaluate the transport of SMZ in biochar treated soils. Biochars were produced from an invasive plant, burcucumber (Sicyos angulatus L.), under slow pyrolysis conditions at peak temperatures of 300 °C (biochar-300) and 700 °C (biochar-700), respectively. The abilities of the biochars to retain SMZ in loamy sand and sandy loam soils were examined under different pHs and SMZ loadings. Soil column experiments were performed with and without biochars addition. Results showed that biochar-700 had a high degree of SMZ retention, with resultant decreased pH in both soils. Modeled effective sorption coefficients (KD,eff) values indicated that the observed high SMZ retention at pH 3 could be attributed to the π-π electron donor-acceptor interaction and electrostatic cation exchange, whereas at pH 5 and 7, cation exchange was the main mechanisms responsible. There was no temporal retardation of SMZ in biochar treated soil as compared to the untreated soil. However, biochar-700 treatment achieved up to 89% and 82% increase in the SMZ retention in sandy loam and loamy sand soils, respectively. The overall results demonstrated that burcucumber biochar produced at higher temperature was effective in reducing the mobility of SMZ in the studied soils.</div></front></TEI><affiliations><list><country><li>Allemagne</li><li>Canada</li><li>Corée du Sud</li><li>République populaire de Chine</li><li>Sri Lanka</li></country><region><li>Rhénanie-Palatinat</li></region><settlement><li>Séoul</li><li>Trèves (Allemagne)</li></settlement><orgName><li>Université de Trèves</li></orgName></list><tree><country name="Sri Lanka"><noRegion><name sortKey="Vithanage, Meththika" sort="Vithanage, Meththika" uniqKey="Vithanage M" first="Meththika" last="Vithanage">Meththika Vithanage</name></noRegion><name sortKey="Rajapaksha, Anushka Upamali" sort="Rajapaksha, Anushka Upamali" uniqKey="Rajapaksha A" first="Anushka Upamali" last="Rajapaksha">Anushka Upamali Rajapaksha</name></country><country name="République populaire de Chine"><noRegion><name sortKey="Tang, Xiangyu" sort="Tang, Xiangyu" uniqKey="Tang X" first="Xiangyu" last="Tang">Xiangyu Tang</name></noRegion></country><country name="Allemagne"><region name="Rhénanie-Palatinat"><name sortKey="Thiele Bruhn, Soren" sort="Thiele Bruhn, Soren" uniqKey="Thiele Bruhn S" first="Sören" last="Thiele-Bruhn">Sören Thiele-Bruhn</name></region></country><country name="Corée du Sud"><noRegion><name sortKey="Kim, Kye Hoon" sort="Kim, Kye Hoon" uniqKey="Kim K" first="Kye Hoon" last="Kim">Kye Hoon Kim</name></noRegion><name sortKey="Lee, Sung Eun" sort="Lee, Sung Eun" uniqKey="Lee S" first="Sung-Eun" last="Lee">Sung-Eun Lee</name></country><country name="Canada"><noRegion><name sortKey="Ok, Yong Sik" sort="Ok, Yong Sik" uniqKey="Ok Y" first="Yong Sik" last="Ok">Yong Sik Ok</name></noRegion></country></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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